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We demonstrate the use of molecular brushes to impart superhydrophilicity to polymer membranes derived from alkylphenol ethoxylate (APEO) surfactants. Films formed by using two polymers with a polyelectrolyte behavior, namely, poly(styrene sulfonate) (PSS) and poly(4-styrenesulfonic acid) (PSAS), which simultaneously form a hydrophilic and water-repellant membrane with the APEO surfactant have high contact angle values of 178° and 162°, respectively. The formation of a stable film is attributed to the attraction of the negatively charged sulfonate groups of PSS to the positively charged surface of the positively charged APEO chain and the solvation of the highly charged sulfonate groups of PSAS in the organic phase by the APEO macromolecular tails in the vicinity of the surface, which prevent the adsorption of water. The highly wettable and, therefore, superhydrophilic membranes show good separation properties (defined by rejection values of 99.97% and 100% for polyethylene glycol (PEG) and bovine serum albumin (BSA), respectively) and high permeability for water vapor. These membranes are used as effective barriers in water separation systems, for example, in pressure-driven membrane distillation systems (P-MD), in which they also show good self-cleaning behavior. These characteristics are promising for applications where self-cleaning and water permeation are required simultaneously. The membrane morphology was characterized by atomic force microscopy and scanning electron 09e8f5149f PowerGREP With Key PowerGREP is a complex software utility designed to help you efficiently search through text and binary files by putting regular expressions at your disposal. It comes loaded with a bunch of advanced options and configuration parameters for experienced users. 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